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A powerful technique to trace the signatures of the first stars is through the metal enrichment in concentrated reservoirs of hydrogen, such as the damped Lyα absorbers (DLAs) in the early Universe. We conducted a survey aimed at discovering DLAs along sight lines to high-z quasars in order to measure element abundances at z > 4. Here we report our first results from this survey for 10 DLAs with redshifts of ≈4.2–5.0. We determine abundances of C, O, Si, S, and Fe, and thereby the metallicities and dust depletions. We find that DLA metallicities at z > 4.5 show a wide diversity spanning ∼3 orders of magnitude. The metallicities of DLAs at 3.7 < z < 5.3 show a larger dispersion compared to that at lower redshifts. Combining our sample with the literature, we find a relatively smooth evolution of metallicity with redshift out to z ∼ 5.3, with a tentative (∼2 sigma) indication of a slight rise in metallicity at 4.5 < z < 5.3. The relative abundances exhibit C enhancement for both metal-poor and metal-enriched DLAs. In addition, α-element enhancement is evident in some DLAs, including a DLA at z = 4.7 with a supersolar metallicity. Comparing [C/O] and [Si/O] with model predictions, four DLAs in our survey seem consistent with a nonzero Population III contribution (three with >~30% Population III contribution). Combining our sample and the literature, we find the dust depletion strength and dust-to-metal ratios to correlate positively with the total (gas+solid phase) metallicity, confirming the presence of metal-rich, dusty DLAs even at ∼1 billion years after the Big Bang. 

Abundances of chemical elements in the interstellar and circumgalactic media of high-redshift galaxies offer important constraints on the nucleosynthesis by early generations of stars. Damped Lyα absorbers (DLAs) in spectra of high-redshift background quasars are excellent sites for obtaining robust measurements of element abundances in distant galaxies. Past studies of DLAs at redshifts z > 4 have measured abundances of 0.01 solar. Here we report the discovery of a DLA at z = 4.7372 with an exceptionally high degree of chemical enrichment. We estimate the H I column density in this absorber to be log (NH I/cm^−2) = 20.48 ± 0.15. Our analysis shows unusually high abundances of carbon and oxygen ([C/H] = 0.88 ± 0.17, [O/H] = 0.71 ± 0.16). Such a high level of enrichment a mere 1.2 Gyr after the Big Bang is surprising because of insufficient time for the required amount of star formation. To our knowledge, this is the first supersolar absorber found at z > 4.5. We find the abundances of Si and Mg to be [Si/H] = -0.56-0.35+0.40 and [Mg/H] = -0.59-0.50+0.27, confirming the metal-rich nature of this absorber. By contrast, Fe shows a much lower abundance ([Fe/H] = -1.53 ± 0.15). We discuss implications of our results for galactic chemical evolution models. The metallicity of this absorber is higher than that of any other known DLA and is >2 orders of magnitude above predictions of chemical evolution models and the NH I-weighted mean metallicity from previous studies at z > 4.5. The relative abundances (e.g., [O/Fe] = 2.29 ± 0.05, [C/Fe] = 2.46 ± 0.08) are also highly unusual compared to predictions for enrichment by early stars. 

The circumgalactic medium (CGM) is a critical repository for metals around galaxies, and serves as the meeting ground for galactic outflows and infalling material from the intergalactic medium. We study the net flow of metals through the CGM in the IllustrisTNG galaxy formation simulations, with a particular focus on the geometry and radial distribution of metal flows. Special care is taken to account for “fuzz” particles, which are often missed by traditional methods of selecting CGM particles in the Illustris simulations, but dominate the net outflow of gas around massive galaxies near the virial radius.